George Tanios, 39, of Morgantown, West Virginia, and Julian Khater, 32, of Pennsylvania, were arrested Sunday.
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The FBI on Tuesday arrested a couple from Owensboro, Kentucky, and a man from Benton, Kentucky for their alleged involvement in the riot.
Investigators say the man was later spotted in the video "carrying a wooden baton in the midst of the large crowd of rioters" near a tunnel that leads into the Capitol.
"Our thoughts and prayers go out to his family, friends, and colleagues," the department said in its statement.